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Epitaxial La0.67Sr0.33MnO3 films grown on orthorhombic NdGaO3 (0 0 1) substrates show predominantly uniaxial magnetic anisotropy. On cooling, we observe the growth of a biaxial contribution, which we quantify by fitting magnetometry data to a coherent rotation model. A film grown under deliberately sub-optimal conditions shows a relatively stronger biaxial contribution that results in a significant population of transverse magnetic domains below ∼200 K, as revealed by photoemission electron microscopy with x-ray magnetic circular dichroism contrast. Care should be taken to avoid these transverse domains in spintronic devices designed to exploit the high low-temperature spin-polarization of La0.67Sr0.33MnO3.
Journal of Physics D: Applied Physics – IOP Publishing
Published: Jan 23, 2013
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