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- Publisher
- Wiley
- Copyright
- © Copyright 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim
- ISSN
- 1438-7492
- eISSN
- 1439-2054
- DOI
- 10.1002/mame.201500425
- Publisher site
- See Article on Publisher Site
Abstract
Mechanically robust and self‐healing rubbers are highly desired to satisfy the increasing demand of high‐performance smart tires and related materials. Herein, a self‐healing rubber nanocomposite with enhanced mechanical and self‐healing performance based on Diels–Alder chemistry has been investigated. The furfuryl grafted styrene‐butadiene rubber and furfuryl terminated MWCNT (MWCNT‐FA) are reacted with bifunctional maleimide to form a covalently bonded and reversibly cross‐linked rubber composite. Obvious reinforcing effect is obtained at high cross‐linking density. Over 200–300% increase in the Young's modulus and toughness can be achieved in the rubber nanocomposites with 5 wt% MWCNT‐FA. Meanwhile, the healing efficiency increased with MWCNT‐FA content. MWCNT‐FA plays dual roles of effective reinforcer and a kind of healant.
Journal
Macromolecular Materials & Engineering – Wiley
Published: May 1, 2016
Keywords: ; ; ; ;