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- Publisher
- Wiley
- Copyright
- Copyright © 2008 American Institute of Chemical Engineers (AIChE)
- ISSN
- 0001-1541
- eISSN
- 1547-5905
- DOI
- 10.1002/aic.11491
- Publisher site
- See Article on Publisher Site
Abstract
The performance of limestone‐derived CaO during many (>1000 in some cases) calcination and carbonation cycles is reported. After 150 cycles, the calcium utilization during carbonation reached a minimum value between 4 and 17%, with the asymptotic level depending strongly on the carbonation time. With the aid of mechanistic studies including investigations on sorbent surface topology by SEM and mercury intrusion, a mechanism for pore evolution during the cyclic capture is proposed consistent with the experimental observations. © 2008 American Institute of Chemical Engineers AIChE J, 2008
Journal
Aiche Journal – Wiley
Published: Jun 1, 2008