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214Bi/214Pb radioactivity ratio in rainwater for residence time estimation of cloud droplets and raindrops

214Bi/214Pb radioactivity ratio in rainwater for residence time estimation of cloud droplets and... Continuous observation of radioactivity ratio of 214Bi to 214Pb as tracers in rainwater was carried out with 15-min cyclic measurement at Nagoya, Japan, from August 2011 to July 2012 to characterise wet deposition. The ratio ranged from 0.55 to 3.82. Based on the observation and a simplified time evolution model of 214Pb and 214Bi radioactivities during rainwater formation, the age of raindrops ranged from sub-10 to several 100 min. The age would have negative correlation to rainfall intensity, but its variation for lower rainfall intensities was quite large. Secular equilibrium of 214Pb and 214Bi radioactivities in cloud water with airborne radon did not hold for some rainfall events. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Radiation Protection Dosimetry Oxford University Press

214Bi/214Pb radioactivity ratio in rainwater for residence time estimation of cloud droplets and raindrops

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References (5)

Publisher
Oxford University Press
Copyright
The Author 2015. Published by Oxford University Press. All rights reserved. For Permissions, please email: journals.permissionsoup.com
ISSN
0144-8420
eISSN
1742-3406
DOI
10.1093/rpd/ncv220
pmid
25911410
Publisher site
See Article on Publisher Site

Abstract

Continuous observation of radioactivity ratio of 214Bi to 214Pb as tracers in rainwater was carried out with 15-min cyclic measurement at Nagoya, Japan, from August 2011 to July 2012 to characterise wet deposition. The ratio ranged from 0.55 to 3.82. Based on the observation and a simplified time evolution model of 214Pb and 214Bi radioactivities during rainwater formation, the age of raindrops ranged from sub-10 to several 100 min. The age would have negative correlation to rainfall intensity, but its variation for lower rainfall intensities was quite large. Secular equilibrium of 214Pb and 214Bi radioactivities in cloud water with airborne radon did not hold for some rainfall events.

Journal

Radiation Protection DosimetryOxford University Press

Published: Nov 24, 2015

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