While a great diversity of rubber/plastic damping blends have been reported, the damping trough resulted from phase incompatibility, which usually exists between the glass transition temperatures (Tg) of each component, remains an unsolved problem by separating the effective temperature range of damping blends. Herein, we reported a new and facile way of preparing rubber/plastic binary blends with high damping property by eliminating the inherent damping trough. Specifically, we envisaged that peroxides can trigger free radical reactions both within and between epoxidized natural rubber/diallyl phthalate prepolymer moieties, which serve as the co‐vulcanizer to generate interphase reactions thus enhancing phase compatibility. Accordingly, apart from the resulting high damping epoxidized natural rubber40/diallyl phthalate prepolymer binary blends with an effective (tan δmin > 0.35) temperature range of 178 °C from −33 to 145 °C, the proposal has also been demonstrated via the support of broadband dielectric spectrometer testing, dynamic mechanical analysis, and differential scanning calorimetry. © 2018 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2018, 135, 46300.
Journal of Applied Polymer Science – Wiley
Published: Jan 15, 2018
Keywords: ; ; ;
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