Vibrational dynamics in liquids studied by non-linear infrared spectroscopy

Vibrational dynamics in liquids studied by non-linear infrared spectroscopy Three-pulse photon echo experiments in the infrared region have been performed to study vibrational dephasing and transition frequency fluctuations in solutions. Time-integrated and frequency-resolved photon echo signals of the –N=C=N– anti-symmetric stretching mode of di-p-tolylcarbodiimide show an oscillatory behavior due to interference with a band nearby. Solvation dynamics or frequency fluctuations of several ions in hydrogen-bonding solvents have been studied and a couple of general trends of the time-correlation function of the frequency fluctuation on these systems have been observed. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Research on Chemical Intermediates Springer Journals

Vibrational dynamics in liquids studied by non-linear infrared spectroscopy

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Publisher
Brill Academic Publishers
Copyright
Copyright © 2005 by VSP
Subject
Chemistry; Inorganic Chemistry; Physical Chemistry; Catalysis
ISSN
0922-6168
eISSN
1568-5675
D.O.I.
10.1163/1568567054909069
Publisher site
See Article on Publisher Site

Abstract

Three-pulse photon echo experiments in the infrared region have been performed to study vibrational dephasing and transition frequency fluctuations in solutions. Time-integrated and frequency-resolved photon echo signals of the –N=C=N– anti-symmetric stretching mode of di-p-tolylcarbodiimide show an oscillatory behavior due to interference with a band nearby. Solvation dynamics or frequency fluctuations of several ions in hydrogen-bonding solvents have been studied and a couple of general trends of the time-correlation function of the frequency fluctuation on these systems have been observed.

Journal

Research on Chemical IntermediatesSpringer Journals

Published: Sep 1, 2005

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