Products formed from alpha radiolysis of chloride brines

Products formed from alpha radiolysis of chloride brines Under alpha irradiation, alkaline chloride brines form H2 (G = 1.2), O2 and chlorate proportional to the dose. The concentrations of additionally formed ClO- and ClO- 2 reach an equilibrium value which depends on the dose rate and the chloride concentration. The solutions become strongly oxidizing (Eh = 900 mV), their pH decreases. This behaviour can be simulated by means of a kinetic model. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Research on Chemical Intermediates Springer Journals

Products formed from alpha radiolysis of chloride brines

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Publisher
Springer Journals
Copyright
Copyright © 2001 by VSP
Subject
Chemistry; Inorganic Chemistry; Physical Chemistry; Catalysis
ISSN
0922-6168
eISSN
1568-5675
D.O.I.
10.1163/156856701104202147
Publisher site
See Article on Publisher Site

Abstract

Under alpha irradiation, alkaline chloride brines form H2 (G = 1.2), O2 and chlorate proportional to the dose. The concentrations of additionally formed ClO- and ClO- 2 reach an equilibrium value which depends on the dose rate and the chloride concentration. The solutions become strongly oxidizing (Eh = 900 mV), their pH decreases. This behaviour can be simulated by means of a kinetic model.

Journal

Research on Chemical IntermediatesSpringer Journals

Published: Jul 1, 2001

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