Under alpha irradiation, alkaline chloride brines form H2 (G = 1.2), O2 and chlorate proportional to the dose. The concentrations of additionally formed ClO- and ClO- 2 reach an equilibrium value which depends on the dose rate and the chloride concentration. The solutions become strongly oxidizing (Eh = 900 mV), their pH decreases. This behaviour can be simulated by means of a kinetic model.
Research on Chemical Intermediates – Springer Journals
Published: Jul 1, 2001
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