Methane activation over zeolite catalysts: The methylation of benzene

Methane activation over zeolite catalysts: The methylation of benzene The methylation of benzene with methane over ZSM-5 zeolite catalysts in a high pressure static reactor is shown to require oxygen as a reactant, implicating methanol as a key intermediate species. In the case of zeolite H-beta, methyl aromatics can be formed in the absence of oxygen, consistent with an earlier report that these products are formed from cracking of benzene over the acid zeolite. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Research on Chemical Intermediates Springer Journals

Methane activation over zeolite catalysts: The methylation of benzene

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Publisher
Brill Academic Publishers
Copyright
Copyright © 2000 by VSP
Subject
Chemistry; Catalysis; Physical Chemistry; Inorganic Chemistry
ISSN
0922-6168
eISSN
1568-5675
D.O.I.
10.1163/156856700X00228
Publisher site
See Article on Publisher Site

Abstract

The methylation of benzene with methane over ZSM-5 zeolite catalysts in a high pressure static reactor is shown to require oxygen as a reactant, implicating methanol as a key intermediate species. In the case of zeolite H-beta, methyl aromatics can be formed in the absence of oxygen, consistent with an earlier report that these products are formed from cracking of benzene over the acid zeolite.

Journal

Research on Chemical IntermediatesSpringer Journals

Published: Jan 1, 2000

References

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