Laser-based measurements of pressure broadening and pressure shift coefficients of combustion-relevant absorption lines in the near-infrared region

Laser-based measurements of pressure broadening and pressure shift coefficients of... A set of high-resolution absorption spectrometers based on TDLAS was used to determine the impact of combustion-relevant gases on the pressure shift and broadening of H2O, CO2, C2H2 and CH4 absorption lines in the near-infrared spectral region. In particular, self- and foreign-broadening coefficients induced by CO2, N2, O2, air, C2H2 and CH4 were measured. The absorption lines under investigation are suitable to measure the respective species in typical combustion environments via laser absorption spectroscopy. Additionally, species-dependent self- and foreign-induced pressure shift coefficients were measured and compared to the literature. The experiments were performed in two specifically designed absorption cells over a wide pressure range from 5 to 180 kPa. Different sources of uncertainty were identified and quantified to achieve relative measurement uncertainties of 0.7–1.5% for broadening coefficients and 0.6–1.6% for pressure shift coefficients. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Applied Physics B Springer Journals

Laser-based measurements of pressure broadening and pressure shift coefficients of combustion-relevant absorption lines in the near-infrared region

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Publisher
Springer Berlin Heidelberg
Copyright
Copyright © 2018 by Springer-Verlag GmbH Germany, part of Springer Nature
Subject
Physics; Physics, general; Physical Chemistry; Optics, Lasers, Photonics, Optical Devices; Quantum Optics; Engineering, general
ISSN
0946-2171
eISSN
1432-0649
D.O.I.
10.1007/s00340-018-6993-y
Publisher site
See Article on Publisher Site

Abstract

A set of high-resolution absorption spectrometers based on TDLAS was used to determine the impact of combustion-relevant gases on the pressure shift and broadening of H2O, CO2, C2H2 and CH4 absorption lines in the near-infrared spectral region. In particular, self- and foreign-broadening coefficients induced by CO2, N2, O2, air, C2H2 and CH4 were measured. The absorption lines under investigation are suitable to measure the respective species in typical combustion environments via laser absorption spectroscopy. Additionally, species-dependent self- and foreign-induced pressure shift coefficients were measured and compared to the literature. The experiments were performed in two specifically designed absorption cells over a wide pressure range from 5 to 180 kPa. Different sources of uncertainty were identified and quantified to achieve relative measurement uncertainties of 0.7–1.5% for broadening coefficients and 0.6–1.6% for pressure shift coefficients.

Journal

Applied Physics BSpringer Journals

Published: May 29, 2018

References

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