Collisional self-broadening coefficients and probabilities of spontaneous emission of the CO2 1000–0001 transition lines

Collisional self-broadening coefficients and probabilities of spontaneous emission of the CO2... Using a tunable frequency-stabilized CO2 laser, the pressure dependences of unsaturated absorption coefficients (AC) are measured in pure carbon dioxide in the pressure range from 5 to 30 Torr, where the spectral line shape is described by the Voigt profile. The absorption coefficients are measured in the centers of R(8), R(22), R(34), P(22), and P(36) spectral lines of the 1000–0001 transition in the temperature range 300–700 K. By means of the least-squares method, the inverse problem is solved for the system of equations for AC at different pressures in the temperature range under study. The self-broadening coefficients $${\gamma _{C{O_2} - C{O_2}}}$$ γ C O 2 − C O 2 and the probabilities of spontaneous emission A ik are derived. A new formula is proposed for $${\gamma _{C{O_2} - C{O_2}}}$$ γ C O 2 − C O 2 (T) dependence. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Atmospheric and Oceanic Optics Springer Journals

Collisional self-broadening coefficients and probabilities of spontaneous emission of the CO2 1000–0001 transition lines

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Publisher
Pleiades Publishing
Copyright
Copyright © 2017 by Pleiades Publishing, Ltd.
Subject
Physics; Optics, Lasers, Photonics, Optical Devices
ISSN
1024-8560
eISSN
2070-0393
D.O.I.
10.1134/S1024856017040030
Publisher site
See Article on Publisher Site

Abstract

Using a tunable frequency-stabilized CO2 laser, the pressure dependences of unsaturated absorption coefficients (AC) are measured in pure carbon dioxide in the pressure range from 5 to 30 Torr, where the spectral line shape is described by the Voigt profile. The absorption coefficients are measured in the centers of R(8), R(22), R(34), P(22), and P(36) spectral lines of the 1000–0001 transition in the temperature range 300–700 K. By means of the least-squares method, the inverse problem is solved for the system of equations for AC at different pressures in the temperature range under study. The self-broadening coefficients $${\gamma _{C{O_2} - C{O_2}}}$$ γ C O 2 − C O 2 and the probabilities of spontaneous emission A ik are derived. A new formula is proposed for $${\gamma _{C{O_2} - C{O_2}}}$$ γ C O 2 − C O 2 (T) dependence.

Journal

Atmospheric and Oceanic OpticsSpringer Journals

Published: Aug 24, 2017

References

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