Bithiazolidinylidene polymers: synthesis and electronic interactions with transition metal dichalcogenidesElectronic supplementary information (ESI) available. See DOI: 10.1039/c8sc01416g

Bithiazolidinylidene polymers: synthesis and electronic interactions with transition metal... We describe the synthesis of electron acceptors consisting of bithiazolidinylidene (BT) derivatives incorporated into solution processible polymers. Novel BT-containing polymers displayed p-doping behavior when in contact with the n-type transition metal dichalcogenide (TMDC) MoS2. A work function (WF) increase of MoS2, resulting from contact with BT polymers, was measured by Kelvin probe force microscopy (KPFM), representing the first example of polymer p-doping of MoS2, which is beneficial for advancing the design of electronically tailored TMDCs. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Chemical Science Royal Society of Chemistry

Bithiazolidinylidene polymers: synthesis and electronic interactions with transition metal dichalcogenidesElectronic supplementary information (ESI) available. See DOI: 10.1039/c8sc01416g

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Publisher
Royal Society of Chemistry
Copyright
This journal is © The Royal Society of Chemistry
ISSN
2041-6520
D.O.I.
10.1039/c8sc01416g
Publisher site
See Article on Publisher Site

Abstract

We describe the synthesis of electron acceptors consisting of bithiazolidinylidene (BT) derivatives incorporated into solution processible polymers. Novel BT-containing polymers displayed p-doping behavior when in contact with the n-type transition metal dichalcogenide (TMDC) MoS2. A work function (WF) increase of MoS2, resulting from contact with BT polymers, was measured by Kelvin probe force microscopy (KPFM), representing the first example of polymer p-doping of MoS2, which is beneficial for advancing the design of electronically tailored TMDCs.

Journal

Chemical ScienceRoyal Society of Chemistry

Published: May 17, 2018

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