Applied Catalysis B: Environmental 235 (2018) 130–142 Contents lists available at ScienceDirect Applied Catalysis B: Environmental journal homepage: www.elsevier.com/locate/apcatb Zeolite–supported nickel phyllosilicate catalyst for CeO hydrogenolysis of cyclic ethers and polyols a,b a a b, Elmira Soghrati , Theodore Kay Chen Ong , Chee Kok Poh , Sibudjing Kawi , a, Armando Borgna Heterogeneous Catalysis Division, Institute of Chemical and Engineering Sciences, Agency for Science, Technology, and Research, 1 Pesek Road, Jurong Island, 627833, Singapore Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, 117585, Singapore ARTIC L E I NF O ABSTRAC T Keywords: In this study, a series of zeolites, including small pore (SAPO–34), medium pore (Ferrierite, ZSM–5, and Hydrogenolysis ZSM–11), and large pore (MOR and BETA) zeolites were explored as supports for nickel catalysts. The catalysts Nickel were prepared by the deposition–precipitation (D–P) method to obtain ca. 10 wt% Ni loading. The structures of Phyllosilicate prepared catalysts were elucidated using a wide range of characterization techniques such as BET, XRD, TEM, Zeolite H –TPR, NH –TPD, FTIR, and XPS. It was found that 1:1 nickel phyllosilicate structures is formed over D–P 2 3 Conﬁnement eﬀect nickel catalysts, while 2:1 nickel phyllosilicate
Applied Catalysis B: Environmental – Elsevier
Published: Nov 5, 2018
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