J. Chem. Thermodynamics 120 (2018) 45–53 Contents lists available at ScienceDirect J. Chem. Thermodynamics journal homepage: www.elsevier.com/locate/jct Solubility and hydrolysis of U(VI) in 0.5 mol/kg NaCl solutions at T = 22 and 80 C a,⇑ a,⇑ b b a Francesco Endrizzi , Xavier Gaona , Maria Marques Fernandes , Bart Baeyens , Marcus Altmaier Karlsruhe Institute of Technology, Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany Paul Scherrer Institute, Laboratory for Waste Management, Villigen PSI, CH-5232, Switzerland article i nfo abstract Article history: In this study, the solubility and hydrolysis of U(VI) was investigated at elevated temperature. Received 31 May 2017 Experiments were performed in solutions of NaCl 0.51 mol/kg of water in the pH range 4–13.4 (with Received in revised form 9 January 2018 + pH = –log[H ]) at T = 22 ± 3 and 80 ± 5 C under N /Ar atmosphere. Two solid phases were used as m 2 Accepted 11 January 2018 starting U(VI) materials: UO 2H O(cr) equilibrated in solutions with 4 pH 5 and Na U O H O(cr) 3 2 m 2 2 7 2 Available online 13 January 2018 (a synthetic clarkeite-like phase) equilibrated in
The Journal of Chemical Thermodynamics – Elsevier
Published: May 1, 2018
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