Polycyclic aromatic hydrocarbons in soils and lichen from the western Tibetan Plateau: Concentration profiles, distribution and its influencing factors

Polycyclic aromatic hydrocarbons in soils and lichen from the western Tibetan Plateau:... The Tibetan Plateau (TP) is a huge area and rarely affected by human activity, and is regarded as one of the most remote regions on the earth. Many studies about the long-range atmospheric transport (LRAT) of semi-volatile organic compounds (SVOCs) were conducted in southern and central TP. However, there are very limited studies focused on PAHs in the western TP and the concentrations profiles, distribution and its controlling factors in this area remains unclear. Thus, to explore this knowledge gap, 37 surface soil samples and 23 lichen samples were collected and analyzed for PAHs. The total concentration of 16 US EPA's priority PAHs (∑16PAHs) in western TP ranges 14.4–59.5ng/g and 38.0–133ng/g dry weight (dw) with a mean value of 30.8 and 84.6ng/g dw in soil and lichen, respectively, which is lower than the concentrations in most remote areas worldwide. In the western TP, low molecular weight PAHs (2–3 rings) are dominant (occupied 77.4% and 87.9% on average in soil and lichen, respectively), implying a significant contribution of LRAT in this area. The significant linear correlations (R2 = 0.372–0.627, p < 0.05) between longitude and soil concentration suggest a strong impact of the westerly wind on the distribution of PAHs in soil. In addition, the concentration ratio of lichen/soil (L/S) was found to linearly increase with the increasing log KOA of individual PAH, suggesting lichen has a strong ability in filtering more lipophilic airborne pollutants in western TP. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Ecotoxicology and Environmental Safety Elsevier

Polycyclic aromatic hydrocarbons in soils and lichen from the western Tibetan Plateau: Concentration profiles, distribution and its influencing factors

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Publisher
Elsevier
Copyright
Copyright © 2018 Elsevier Inc.
ISSN
0147-6513
eISSN
1090-2414
D.O.I.
10.1016/j.ecoenv.2018.01.009
Publisher site
See Article on Publisher Site

Abstract

The Tibetan Plateau (TP) is a huge area and rarely affected by human activity, and is regarded as one of the most remote regions on the earth. Many studies about the long-range atmospheric transport (LRAT) of semi-volatile organic compounds (SVOCs) were conducted in southern and central TP. However, there are very limited studies focused on PAHs in the western TP and the concentrations profiles, distribution and its controlling factors in this area remains unclear. Thus, to explore this knowledge gap, 37 surface soil samples and 23 lichen samples were collected and analyzed for PAHs. The total concentration of 16 US EPA's priority PAHs (∑16PAHs) in western TP ranges 14.4–59.5ng/g and 38.0–133ng/g dry weight (dw) with a mean value of 30.8 and 84.6ng/g dw in soil and lichen, respectively, which is lower than the concentrations in most remote areas worldwide. In the western TP, low molecular weight PAHs (2–3 rings) are dominant (occupied 77.4% and 87.9% on average in soil and lichen, respectively), implying a significant contribution of LRAT in this area. The significant linear correlations (R2 = 0.372–0.627, p < 0.05) between longitude and soil concentration suggest a strong impact of the westerly wind on the distribution of PAHs in soil. In addition, the concentration ratio of lichen/soil (L/S) was found to linearly increase with the increasing log KOA of individual PAH, suggesting lichen has a strong ability in filtering more lipophilic airborne pollutants in western TP.

Journal

Ecotoxicology and Environmental SafetyElsevier

Published: May 15, 2018

References

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