Performance and degradation mechanisms of CLC particles produced by industrial methods

Performance and degradation mechanisms of CLC particles produced by industrial methods Fuel 216 (2018) 71–82 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Performance and degradation mechanisms of CLC particles produced by industrial methods a, a a a a Arnold Lambert , Airy Tilland , William Pelletant , Stéphane Bertholin , Florent Moreau , a b Isabelle Clemençon , Mahdi Yazdanpanah IFP Energies nouvelles, BP3, 69360 Solaize, France Total, Research & Technology Gonfreville (TRTG), 76700 Harfleur, France GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: A promising copper based oxygen carrier produced using industrially-relevant manufacturing equipment has Chemical looping combustion been aged in IFPEN’s10 kW Chemical Looping Combustion pilot plant. Methane combustion was performed at th Oxygen carrier ageing 900 °C for 160 h with an OC/fuel ratio of 1.2. While full methane conversion to CO and water was achieved in CuO/Al O 2 3 the early stage of the experiment, fast deactivation was observed. The oxygen carrying particles were thoroughly Degradation mechanisms characterized at various stages of the ageing experiment, from which a pathway leading to deactivation is proposed. 1. Introduction penalty. The process relies on circulating metal oxides which act as oxygen carriers (OC) between an oxidation and a reduction reactor [2]. In http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Fuel Elsevier

Performance and degradation mechanisms of CLC particles produced by industrial methods

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Publisher
Elsevier
Copyright
Copyright © 2017 Elsevier Ltd
ISSN
0016-2361
D.O.I.
10.1016/j.fuel.2017.11.115
Publisher site
See Article on Publisher Site

Abstract

Fuel 216 (2018) 71–82 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Performance and degradation mechanisms of CLC particles produced by industrial methods a, a a a a Arnold Lambert , Airy Tilland , William Pelletant , Stéphane Bertholin , Florent Moreau , a b Isabelle Clemençon , Mahdi Yazdanpanah IFP Energies nouvelles, BP3, 69360 Solaize, France Total, Research & Technology Gonfreville (TRTG), 76700 Harfleur, France GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: A promising copper based oxygen carrier produced using industrially-relevant manufacturing equipment has Chemical looping combustion been aged in IFPEN’s10 kW Chemical Looping Combustion pilot plant. Methane combustion was performed at th Oxygen carrier ageing 900 °C for 160 h with an OC/fuel ratio of 1.2. While full methane conversion to CO and water was achieved in CuO/Al O 2 3 the early stage of the experiment, fast deactivation was observed. The oxygen carrying particles were thoroughly Degradation mechanisms characterized at various stages of the ageing experiment, from which a pathway leading to deactivation is proposed. 1. Introduction penalty. The process relies on circulating metal oxides which act as oxygen carriers (OC) between an oxidation and a reduction reactor [2]. In

Journal

FuelElsevier

Published: Mar 15, 2018

References

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