Fuel 216 (2018) 71–82 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Performance and degradation mechanisms of CLC particles produced by industrial methods a, a a a a Arnold Lambert , Airy Tilland , William Pelletant , Stéphane Bertholin , Florent Moreau , a b Isabelle Clemençon , Mahdi Yazdanpanah IFP Energies nouvelles, BP3, 69360 Solaize, France Total, Research & Technology Gonfreville (TRTG), 76700 Harﬂeur, France GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: A promising copper based oxygen carrier produced using industrially-relevant manufacturing equipment has Chemical looping combustion been aged in IFPEN’s10 kW Chemical Looping Combustion pilot plant. Methane combustion was performed at th Oxygen carrier ageing 900 °C for 160 h with an OC/fuel ratio of 1.2. While full methane conversion to CO and water was achieved in CuO/Al O 2 3 the early stage of the experiment, fast deactivation was observed. The oxygen carrying particles were thoroughly Degradation mechanisms characterized at various stages of the ageing experiment, from which a pathway leading to deactivation is proposed. 1. Introduction penalty. The process relies on circulating metal oxides which act as oxygen carriers (OC) between an oxidation and a reduction reactor . In
Fuel – Elsevier
Published: Mar 15, 2018
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