Journal of Catalysis 360 (2018) 127–134 Contents lists available at ScienceDirect Journal of Catalysis journal homepage: www.elsevier.com/locate/jcat One-pot monoterpene alcohol amination over Au/ZrO catalyst: Effect of the substrate structure a,b c a,b,⇑ c c b,c Yu. S. Demidova , E.V. Suslov , I.L. Simakova , E.S. Mozhajcev , D.V. Korchagina , K.P. Volcho , b,c d e N.F. Salakhutdinov , A. Simakov , D. Yu. Murzin Boreskov Institute of Catalysis, pr. Lavrentieva 5, 630090 Novosibirsk, Russia Novosibirsk State University, Pirogova 2, 630090 Novosibirsk, Russia Novosibirsk Institute of Organic Chemistry, pr. Lavrentieva 9, 630090 Novosibirsk, Russia Universidad Nacional Autónoma de México, Centro de Nanociencias y Nanotecnología, km. 107 carretera Tijuana a Ensenada, C.P. 22860 Ensenada, BC, México Process Chemistry Centre, Åbo Akademi University, Biskopsgatan 8, FI-20500 Turku/Åbo, Finland article i nfo abstract Article history: One-pot amination of natural monoterpene alcohols was studied over Au/ZrO catalyst, focusing on the Received 13 December 2017 structure effect of substrates selected based on their pharmaceutical relevance. Bicyclic (myrtenol and Revised 17 January 2018 nopol, bearing an unconjugated –OH group) and monocyclic (perillyl) alcohols were chosen for aniline Accepted 19 January 2018 amination under comparable conditions. Utilization of nopol resulted in a tenfold decrease in
Journal of Catalysis – Elsevier
Published: Apr 1, 2018
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