Chemical Engineering Journal 336 (2018) 721–731 Contents lists available at ScienceDirect Chemical Engineering Journal journal homepage: www.elsevier.com/locate/cej Non-radical-dominated catalytic degradation of bisphenol A by ZIF-67 derived nitrogen-doped carbon nanotubes frameworks in the presence of peroxymonosulfate ⁎ ⁎ Wenjie Ma, Na Wang, Yanan Fan, Tianze Tong, Xijiang Han , Yunchen Du MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, China GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: Nitrogen-doped carbon materials have been one of the most remarkable families of materials with promising ZIF-67 applications in many ﬁelds. In this study, a series of nitrogen-doped carbon nanotubes frameworks (NCNTFs) Nitrogen-doped carbon nanotubes with distinguishable nitrogen content and graphitization degree have been successfully prepared through in situ Peroxymonosulfate transformation of ZIF-67 under N /H atmosphere at diﬀerent pyrolysis temperature. Compared with conven- 2 2 Bisphenol A degradation tional nitrogen-doped carbon materials derived from metal-organic frameworks, the formation of intertwined Non-radical process carbon nanotubes harvests desirable mesoporous structure that is favorable for the mass transfer and diﬀusion of reaction substances. When they are applied for catalytic degradation of Bisphenol A (BPA) in the presence
Chemical Engineering Journal – Elsevier
Published: Mar 15, 2018
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