Fuel 217 (2018) 106–110 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Large volume in situ H production on ﬁxed bed reactor by concentrated formic acid aqueous solution Yaqiu Tao, Lulu Tao, Zhigang Pan , Simin Qiu, Xiaodong Shen College of Materials Science and Engineering, Nanjing Tech University, 5 Xinmofan Road, Nanjing, Jiangsu Province 21009, PR China GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: Formic acid is a promising hydrogen storage material for its high H capacity, easy transfer and moderate H 2 2 Formic acid regeneration conditions. Active carbon supported Mo C with or without Co doping were used as the hetero- Mo C geneous catalyst in the decomposition of a high concentrated aqueous solution of formic acid up to 50% on a Hydrogen production ﬁxed bed reactor. For a given ﬂow rate and reaction temperature, though higher volume of H is produced per unit time, the increase in formic acid’s concentration reduces both H selectivity and formic acid conversion rate. At 250 °C, a stream of 236 mL/min H was generated continuously at a high H selectivity (91%) and formic acid 2 2 conversion rate (86%), from a 10% formic acid
Fuel – Elsevier
Published: Apr 1, 2018
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