Large volume in situ H2 production on fixed bed reactor by concentrated formic acid aqueous solution

Large volume in situ H2 production on fixed bed reactor by concentrated formic acid aqueous solution Fuel 217 (2018) 106–110 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Large volume in situ H production on fixed bed reactor by concentrated formic acid aqueous solution Yaqiu Tao, Lulu Tao, Zhigang Pan , Simin Qiu, Xiaodong Shen College of Materials Science and Engineering, Nanjing Tech University, 5 Xinmofan Road, Nanjing, Jiangsu Province 21009, PR China GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: Formic acid is a promising hydrogen storage material for its high H capacity, easy transfer and moderate H 2 2 Formic acid regeneration conditions. Active carbon supported Mo C with or without Co doping were used as the hetero- Mo C geneous catalyst in the decomposition of a high concentrated aqueous solution of formic acid up to 50% on a Hydrogen production fixed bed reactor. For a given flow rate and reaction temperature, though higher volume of H is produced per unit time, the increase in formic acid’s concentration reduces both H selectivity and formic acid conversion rate. At 250 °C, a stream of 236 mL/min H was generated continuously at a high H selectivity (91%) and formic acid 2 2 conversion rate (86%), from a 10% formic acid http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Fuel Elsevier

Large volume in situ H2 production on fixed bed reactor by concentrated formic acid aqueous solution

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Publisher
Elsevier
Copyright
Copyright © 2017 Elsevier Ltd
ISSN
0016-2361
D.O.I.
10.1016/j.fuel.2017.12.011
Publisher site
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Abstract

Fuel 217 (2018) 106–110 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Large volume in situ H production on fixed bed reactor by concentrated formic acid aqueous solution Yaqiu Tao, Lulu Tao, Zhigang Pan , Simin Qiu, Xiaodong Shen College of Materials Science and Engineering, Nanjing Tech University, 5 Xinmofan Road, Nanjing, Jiangsu Province 21009, PR China GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: Formic acid is a promising hydrogen storage material for its high H capacity, easy transfer and moderate H 2 2 Formic acid regeneration conditions. Active carbon supported Mo C with or without Co doping were used as the hetero- Mo C geneous catalyst in the decomposition of a high concentrated aqueous solution of formic acid up to 50% on a Hydrogen production fixed bed reactor. For a given flow rate and reaction temperature, though higher volume of H is produced per unit time, the increase in formic acid’s concentration reduces both H selectivity and formic acid conversion rate. At 250 °C, a stream of 236 mL/min H was generated continuously at a high H selectivity (91%) and formic acid 2 2 conversion rate (86%), from a 10% formic acid

Journal

FuelElsevier

Published: Apr 1, 2018

References

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