10.1016/j.apenergy.2018.05.082

10.1016/j.apenergy.2018.05.082 Applied Energy 225 (2018) 912–921 Contents lists available at ScienceDirect Applied Energy journal homepage: www.elsevier.com/locate/apenergy Effects of supports on reduction activity and carbon deposition of iron oxide for methane chemical looping hydrogen generation Min Zhu, Shiyi Chen, Ahsanullah Soomro, Jun Hu, Zhao Sun, Shiwei Ma, Wenguo Xiang Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing, China HIG HLI GHTS Carbon resistance of oxygen carrier was enhanced by inner supports. Four supports MgAl O , CeO , ZrO , and CeZrO were combined with iron oxide. 2 4 2 2 4 Reduction activity is related to the surface area of oxygen carriers. Carbon resistance depends on the oxygen transfer capacity. Oxidation of deposited carbon causes oxygen carrier sintering. ARTIC L E I NF O ABSTRAC T Keywords: Chemical looping hydrogen generation is a promising technology which has the potential to efficiently produce Iron-based oxygen carriers hydrogen and capture CO with the aid of iron-based oxygen carriers. The properties of the iron-based oxygen Chemical looping hydrogen generation carrier, such as carbon resistance, redox activity, and cycle stability, are critical factors for the development of Carbon deposition CLHG process. In http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png

10.1016/j.apenergy.2018.05.082

Elsevier — Jun 11, 2020

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Abstract

Applied Energy 225 (2018) 912–921 Contents lists available at ScienceDirect Applied Energy journal homepage: www.elsevier.com/locate/apenergy Effects of supports on reduction activity and carbon deposition of iron oxide for methane chemical looping hydrogen generation Min Zhu, Shiyi Chen, Ahsanullah Soomro, Jun Hu, Zhao Sun, Shiwei Ma, Wenguo Xiang Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing, China HIG HLI GHTS Carbon resistance of oxygen carrier was enhanced by inner supports. Four supports MgAl O , CeO , ZrO , and CeZrO were combined with iron oxide. 2 4 2 2 4 Reduction activity is related to the surface area of oxygen carriers. Carbon resistance depends on the oxygen transfer capacity. Oxidation of deposited carbon causes oxygen carrier sintering. ARTIC L E I NF O ABSTRAC T Keywords: Chemical looping hydrogen generation is a promising technology which has the potential to efficiently produce Iron-based oxygen carriers hydrogen and capture CO with the aid of iron-based oxygen carriers. The properties of the iron-based oxygen Chemical looping hydrogen generation carrier, such as carbon resistance, redox activity, and cycle stability, are critical factors for the development of Carbon deposition CLHG process. In

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