•We reported direct formation of bilayer films without surface modification on PLA films.•This study opens a promising route to form bilayer architecture to create synergism.•The release profiles of thymol from bilayer films were well fitted with Fick’s second law.•PLA layer limited thymol release and bilayer films possessed directional releasing role.
Carbohydrate Polymers – Elsevier
Published: Feb 1, 2018
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