Fuel 216 (2018) 245–254 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Full Length Article Ce Zr O solid solutions for catalytic synthesis of dimethyl carbonate x 1−x 2 from CO : Reaction mechanism and the eﬀect of catalyst morphology on catalytic activity a a b a, Ashif H. Tamboli , Avinash A. Chaugule , Suresh W. Gosavi , Hern Kim Department of Energy Science and Technology, Smart Living Innovation Technology Center, Myongji University, Yongin, Gyeonggi-do 17058, Republic of Korea Department of Physics, Savitribai Phule, Pune University, Pune, Maharashtra, India GR APHICAL A BSTRACT ARTICLE I NFO ABSTRACT Keywords: In the development of green and sustainable processes, one-pot conversion of carbon dioxide into value-added Ceria-zirconia organic chemicals such as dimethyl carbonate (DMC) attracted much attention. In the present study, a series of Solid solutions Ce Zr O solid solutions (x = 0.25, 0.5, 0.75) having acid/base and high surface area was synthesized for x 1−x 2 Formation mechanism eﬃcient production of DMC from CO and methanol. The as-prepared catalyst was characterized by scanning Carbon dioxide electron microscopy (SEM), high-resolution transmission electron microscope (HRTEM), Fourier-transform in- Dimethyl carbonate frared spectroscopy (FTIR), X-ray diﬀraction (XRD), X-ray photoelectron spectroscopy (XPS) and
Fuel – Elsevier
Published: Mar 15, 2018
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