Catalytic carpets: Pt@MIL-101@electrospun PCL, a surprisingly active and robust hydrogenation catalyst

Catalytic carpets: Pt@MIL-101@electrospun PCL, a surprisingly active and robust hydrogenation... Journal of Catalysis 360 (2018) 81–88 Contents lists available at ScienceDirect Journal of Catalysis journal homepage: www.elsevier.com/locate/jcat Catalytic carpets: Pt@MIL-101@electrospun PCL, a surprisingly active and robust hydrogenation catalyst a,⇑,1 a,1 a,b c c Karen Leus , Chidharth Krishnaraj , Luca Verhoeven , Véronique Cremers , Jolien Dendooven , c b a,⇑ Ranjith K. Ramachandran , Peter Dubruel , Pascal Van Der Voort Department of Chemistry, Centre for Ordered Materials, Organometallics and Catalysis (COMOC), Ghent University, Krijgslaan 281-S3, 9000 Ghent, Belgium Department of Macromolecular and Organic Chemistry, Polymer Chemistry and Biomaterials Group, Ghent University, Krijgslaan 281-S4, 9000 Ghent, Belgium Department of Solid State Sciences, Conformal Coatings on Nanomaterials (CoCooN), Ghent University, Krijgslaan 281-S1, 9000 Ghent, Belgium article i nfo abstract Article history: Metal Organic Frameworks (MOFs) have been explored widely to create heterogeneity in a catalytic sys- Received 30 November 2017 tem. Catalytic applications require the use of stable catalysts with no leaching and easy recovery. In this Revised 19 January 2018 regard, Pt@MIL-101 is embedded in a poly-є-caprolactone (PCL) matrix by means of electrospinning to cre- Accepted 20 January 2018 ate a ‘‘catalytic carpet” which is highly efficient and can be recovered within seconds after catalysis. The Available online http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Journal of Catalysis Elsevier

Catalytic carpets: Pt@MIL-101@electrospun PCL, a surprisingly active and robust hydrogenation catalyst

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Publisher
Elsevier
Copyright
Copyright © 2018 Elsevier Inc.
ISSN
0021-9517
D.O.I.
10.1016/j.jcat.2018.01.018
Publisher site
See Article on Publisher Site

Abstract

Journal of Catalysis 360 (2018) 81–88 Contents lists available at ScienceDirect Journal of Catalysis journal homepage: www.elsevier.com/locate/jcat Catalytic carpets: Pt@MIL-101@electrospun PCL, a surprisingly active and robust hydrogenation catalyst a,⇑,1 a,1 a,b c c Karen Leus , Chidharth Krishnaraj , Luca Verhoeven , Véronique Cremers , Jolien Dendooven , c b a,⇑ Ranjith K. Ramachandran , Peter Dubruel , Pascal Van Der Voort Department of Chemistry, Centre for Ordered Materials, Organometallics and Catalysis (COMOC), Ghent University, Krijgslaan 281-S3, 9000 Ghent, Belgium Department of Macromolecular and Organic Chemistry, Polymer Chemistry and Biomaterials Group, Ghent University, Krijgslaan 281-S4, 9000 Ghent, Belgium Department of Solid State Sciences, Conformal Coatings on Nanomaterials (CoCooN), Ghent University, Krijgslaan 281-S1, 9000 Ghent, Belgium article i nfo abstract Article history: Metal Organic Frameworks (MOFs) have been explored widely to create heterogeneity in a catalytic sys- Received 30 November 2017 tem. Catalytic applications require the use of stable catalysts with no leaching and easy recovery. In this Revised 19 January 2018 regard, Pt@MIL-101 is embedded in a poly-є-caprolactone (PCL) matrix by means of electrospinning to cre- Accepted 20 January 2018 ate a ‘‘catalytic carpet” which is highly efficient and can be recovered within seconds after catalysis. The Available online

Journal

Journal of CatalysisElsevier

Published: Apr 1, 2018

References

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