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Yanbo Liu, Guifang Wu, L. Gu (2008)
Enzymatic Treatment of PET Fabrics for Improved HydrophilicityAatcc Review, 8
K. Jaeger, S. Ransac, B. Dijkstra, C. Colson (1994)
Bacterial lipases, 15
Y. Hsieh, L. Cram (1998)
Enzymatic Hydrolysis to Improve Wetting and Absorbency of Polyester FabricsTextile Research Journal, 68
Kasturi Dutta, Shampa Sen, V. Veeranki (2009)
Production, characterization and applications of microbial cutinasesProcess Biochemistry, 44
Stefan Liebminger, A. Eberl, F. Sousa, S. Heumann, G. Fischer-Colbrie, A. Cavaco‐Paulo, G. Guebitz (2007)
Hydrolysis of PET and bis-(benzoyloxyethyl) terephthalate with a new polyesterase from Penicillium citrinumBiocatalysis and Biotransformation, 25
M. Gouda, I. Kleeberg, J. Heuvel, R. Müller, W. Deckwer (2002)
Production of a Polyester Degrading Extracellular Hydrolase from Thermomonospora fuscaBiotechnology Progress, 18
C. Carvalho, M. Aires-Barros, J. Cabral (1999)
Cutinase: from molecular level to bioprocess development.Biotechnology and bioengineering, 66 1
T. Brueckner, A. Eberl, S. Heumann, M. Rabe, G. Guebitz (2008)
Enzymatic and chemical hydrolysis of poly(ethylene terephthalate) fabricsJournal of Polymer Science Part A, 46
E. Almansa, S. Heumann, A. Eberl, G. Fischer-Colbrie, L. Martínková, J. Marek, A. Cavaco‐Paulo, G. Guebitz (2008)
Enzymatic surface hydrolysis of PET enhances bonding in PVC coatingBiocatalysis and Biotransformation, 26
(2004)
Modification of textile fibres by laccase
Mikael Vertommen, V. Nierstrasz, M. Veer, M. Warmoeskerken (2005)
Enzymatic surface modification of poly(ethylene terephthalate).Journal of biotechnology, 120 4
Åsa Ronkvist, Wenchun Xie, Wenhua Lu, R. Gross (2009)
Cutinase-Catalyzed Hydrolysis of Poly(ethylene terephthalate)Macromolecules, 42
Sheng Chen, X. Tong, R. Woodard, G. Du, Jing Wu, Jian Chen (2008)
Identification and Characterization of Bacterial Cutinase*Journal of Biological Chemistry, 283
Jaeger (1994)
10.1111/j.1574-6976.1994.tb00121.xFEMS Microbiol. Rev., 15
Sheng Chen, Lingqia Su, S. Billig, W. Zimmermann, Jian Chen, Jing Wu (2010)
Biochemical characterization of the cutinases from Thermobifida fuscaJournal of Molecular Catalysis B-enzymatic, 63
Thidarat Nimchua, H. Punnapayak, W. Zimmermann (2007)
Comparison of the hydrolysis of polyethylene terephthalate fibers by a hydrolase from Fusarium oxysporum LCH I and Fusarium solani f. sp. pisi.Biotechnology journal, 2 3
H. Kontkanen, M. Saloheimo, J. Péré, A. Miettinen-Oinonen, T. Reinikainen (2006)
Characterization of Melanocarpus albomyces steryl esterase produced in Trichoderma reesei and modification of fibre products with the enzymeApplied Microbiology and Biotechnology, 72
Gangqiang He, G. Huo, Liming Liu, Yang Zhu, G. Du, Jian Chen (2009)
Enhanced cutinase production of Thermobifida fusca by a two-stage batch and fed-batch cultivation strategyBiotechnology and Bioprocess Engineering, 14
A. Feuerhack, M. Alisch-Mark, A. Kisner, S. Pezzin, W. Zimmermann, J. Andreaus (2008)
Biocatalytic surface modification of knitted fabrics made of poly (ethylene terephthalate) with hydrolytic enzymes from Thermobifida fusca KW3bBiocatalysis and Biotransformation, 26
Yoon M. (2002)
Enzymatic modification of polyester.AATCC Rev., 2
M. Alisch-Mark, A. Herrmann, W. Zimmermann (2006)
Increase of the Hydrophilicity of Polyethylene Terephthalate Fibres by Hydrolases from Thermomonospora fusca and Fusarium solani f. sp. pisiBiotechnology Letters, 28
K. Pang, R. Kotek, A. Tonelli (2006)
Review of conventional and novel polymerization processes for polyestersProgress in Polymer Science, 31
R. Müller, H. Schrader, J. Profe, Karolin Dresler, W. Deckwer (2005)
Enzymatic Degradation of Poly(ethylene terephthalate): Rapid Hydrolyse using a Hydrolase from T. fuscaMacromolecular Rapid Communications, 26
C. Carvalho, M. Aires-Barros, J. Cabral (1998)
Cutinase structure, function and biocatalytic applicationsElectronic Journal of Biotechnology, 1
Carla Silva, F. Carneiro, Alexandre O’Neill, L. Fonseca, J. Cabral, G. Guebitz, A. Cavaco‐Paulo (2005)
Cutinase—A new tool for biomodification of synthetic fibersJournal of Polymer Science Part A, 43
A. Eberl, S. Heumann, R. Kotek, F. Kaufmann, S. Mitsche, A. Cavaco-Paulo, G. Gübitz (2008)
Enzymatic hydrolysis of PTT polymers and oligomers.Journal of biotechnology, 135 1
Ping Wang, Qiang Wang, X. Fan, L. Cui, J. Yuan, Sheng Chen, Jing Wu (2009)
Effects of cutinase on the enzymatic shrink-resist finishing of wool fabricsEnzyme and Microbial Technology, 44
A. Eberl, S. Heumann, Tina Brueckner, R. Araújo, A. Cavaco‐Paulo, F. Kaufmann, W. Kroutil, G. Guebitz (2009)
Enzymatic surface hydrolysis of poly(ethylene terephthalate) and bis(benzoyloxyethyl) terephthalate by lipase and cutinase in the presence of surface active molecules.Journal of biotechnology, 143 3
I. Kleeberg, K. Welzel, J. Vandenheuvel, R. Müller, W. Deckwer (2005)
Characterization of a new extracellular hydrolase from Thermobifida fusca degrading aliphatic-aromatic copolyesters.Biomacromolecules, 6 1
Carvalho (1998)
10.2225/vol1-issue3-fulltext-8Electron. J. Biotechnol., 1
I. Donelli, P. Taddei, P. Smet, D. Poelman, V. Nierstrasz, G. Freddi (2009)
Enzymatic surface modification and functionalization of PET: A water contact angle, FTIR, and fluorescence spectroscopy studyBiotechnology and Bioengineering, 103
Carla Silva, A. Cavaco‐Paulo (2008)
Biotransformations in synthetic fibresBiocatalysis and Biotransformation, 26
R. Araújo, Carla Silva, Alexandre O’Neill, N. Micaêlo, G. Guebitz, C. Soares, M. Casal, A. Cavaco‐Paulo (2007)
Tailoring cutinase activity towards polyethylene terephthalate and polyamide 6,6 fibers.Journal of biotechnology, 128 4
M. Alisch, Andreas Feuerhack, H. Müller, B. Mensak, J. Andreaus, Wolfgang Zimmermann (2004)
Biocatalytic modification of polyethylene terephthalate fibres by esterases from actinomycete isolatesBiocatalysis and Biotransformation, 22
X. Wang, D. Lu, L. Jönsson, Feng Hong (2008)
Preparation of a PET‐Hydrolyzing Lipase from Aspergillus oryzae by the Addition of Bis(2‐hydroxyethyl) Terephthalate to the Culture Medium and Enzymatic Modification of PET FabricsEngineering in Life Sciences, 8
Alexandre O’Neill, A. Cavaco‐Paulo (2004)
Monitoring biotransformations in polyestersBiocatalysis and Biotransformation, 22
H. Kim, W. Song (2006)
Lipase treatment of polyester fabricsFibers and Polymers, 7
W. Fett, H. Gérard, R. Moreau, S. Osman, L. Jones (1992)
Cutinase production byStreptomyces spp.Current Microbiology, 25
D. Parikh, T. Calamari, D. Peterson, T. Vigo, W. Goynes, T. Saunders (2002)
FR/resilient perpendicular-laid nonwovens containinq cottonAatcc Review, 2
A bacterial cutinase from Thermobifida fusca, named Tfu_0883, was genetically modified by site‐directed mutagenesis to enhance its activity on poly(ethylene terephthalate) (PET). The new mutations tailored the catalytic site for PET, increasing the affinity of cutinase to this hydrophobic substrate and the ability to hydrolyze it. The mutation I218A was designed to create space and the double mutation Q132A/T101A was designed both to create space and to increase hydrophobicity. The activity of the double mutant on the soluble substrate p‐nitrophenyl butyrate increased two‐fold compared to wild‐type cutinase, while on PET both single and double mutants exhibited considerably higher hydrolysis efficiency. The replacement of specific amino acids at the active site was an effective approach for the improvement of the Tfu_0883 cutinase capacity to hydrolyze polyester surfaces. Thus, this study provides valuable insight on how the function and stability of enzymes can be improved by molecular engineering for their application in synthetic fiber biotransformation.
Biotechnology Journal – Wiley
Published: Oct 1, 2011
Keywords: ; ; ; ;
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