Sublattice site dependence of local electronic states in superstructures of CO built on a Cu(111) surface

Sublattice site dependence of local electronic states in superstructures of CO built on a Cu(111)... A two-dimensional electron gas interacting with an external periodic potential attracts attention as a designable artificial material to explore topological phases. Here, to introduce a periodic potential into a Shockley state, superstructures of CO molecules have been fabricated on a Cu(111) surface by atom manipulation with a low-temperature scanning tunneling microscope. Local electronic states have been investigated in relation to specific locations on the CO triangular lattice. All tunneling spectra of the lattice exhibit a reduction at the bottom energy of the surface-state band, which reflects absorption of surface-state electrons into the bulk. For an (8×8) CO structure, spectra measured at positions corresponding to two equivalent triangular sublattices of artificial graphene have different features near the Fermi level. This sublattice site dependence is not observed for a (6×6) structure. First-principles calculations for a (4×4) structure have reproduced the local density of states that depend on the sublattice sites. These results can be understood that coupling between the surface state and the bulk is strengthened via scattering by the adsorbates, and that the external periodic potential is perturbed by the second layer of the Cu(111) substrate. The periodicity of the external potential appears to be the key parameter which dominates the equivalence of pseudospin states in the artificial graphene. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Physical Review B American Physical Society (APS)

Sublattice site dependence of local electronic states in superstructures of CO built on a Cu(111) surface

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Sublattice site dependence of local electronic states in superstructures of CO built on a Cu(111) surface

Abstract

A two-dimensional electron gas interacting with an external periodic potential attracts attention as a designable artificial material to explore topological phases. Here, to introduce a periodic potential into a Shockley state, superstructures of CO molecules have been fabricated on a Cu(111) surface by atom manipulation with a low-temperature scanning tunneling microscope. Local electronic states have been investigated in relation to specific locations on the CO triangular lattice. All tunneling spectra of the lattice exhibit a reduction at the bottom energy of the surface-state band, which reflects absorption of surface-state electrons into the bulk. For an (8×8) CO structure, spectra measured at positions corresponding to two equivalent triangular sublattices of artificial graphene have different features near the Fermi level. This sublattice site dependence is not observed for a (6×6) structure. First-principles calculations for a (4×4) structure have reproduced the local density of states that depend on the sublattice sites. These results can be understood that coupling between the surface state and the bulk is strengthened via scattering by the adsorbates, and that the external periodic potential is perturbed by the second layer of the Cu(111) substrate. The periodicity of the external potential appears to be the key parameter which dominates the equivalence of pseudospin states in the artificial graphene.
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Publisher
American Physical Society (APS)
Copyright
Copyright © ©2017 American Physical Society
ISSN
1098-0121
eISSN
1550-235X
D.O.I.
10.1103/PhysRevB.96.035424
Publisher site
See Article on Publisher Site

Abstract

A two-dimensional electron gas interacting with an external periodic potential attracts attention as a designable artificial material to explore topological phases. Here, to introduce a periodic potential into a Shockley state, superstructures of CO molecules have been fabricated on a Cu(111) surface by atom manipulation with a low-temperature scanning tunneling microscope. Local electronic states have been investigated in relation to specific locations on the CO triangular lattice. All tunneling spectra of the lattice exhibit a reduction at the bottom energy of the surface-state band, which reflects absorption of surface-state electrons into the bulk. For an (8×8) CO structure, spectra measured at positions corresponding to two equivalent triangular sublattices of artificial graphene have different features near the Fermi level. This sublattice site dependence is not observed for a (6×6) structure. First-principles calculations for a (4×4) structure have reproduced the local density of states that depend on the sublattice sites. These results can be understood that coupling between the surface state and the bulk is strengthened via scattering by the adsorbates, and that the external periodic potential is perturbed by the second layer of the Cu(111) substrate. The periodicity of the external potential appears to be the key parameter which dominates the equivalence of pseudospin states in the artificial graphene.

Journal

Physical Review BAmerican Physical Society (APS)

Published: Jul 19, 2017

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