Separation of two attractive ferromagnetic ellipsoidal particles by hydrodynamic interactions under alternating magnetic field

Separation of two attractive ferromagnetic ellipsoidal particles by hydrodynamic interactions... In applications where magnetic particles are used to detect and dose targeted molecules, it is of major importance to prevent particle clustering and aggregation during the capture stage in order to maximize the capture rate. Elongated ferromagnetic particles can be more interesting than spherical ones due to their large magnetic moment, which facilitates their separation by magnets or the detection by optical measurement of their orientation relaxation time. Under alternating magnetic field, the rotational dynamics of elongated ferromagnetic particles results from the balance between magnetic torque that tends to align the particle axis with the field direction and viscous torque. As for their translational motion, it results from a competition between direct magnetic particle-particle interactions and solvent-flow-mediated hydrodynamic interactions. Due to particle anisotropy, this may lead to intricate translation-rotation couplings. Using numerical simulations and theoretical modeling of the system, we show that two ellipsoidal magnetic particles, initially in a head-to-tail attractive configuration resulting from their remnant magnetization, can repel each other due to hydrodynamic interactions when alternating field is operated. The separation takes place in a range of low frequencies fc1<f<fc2. The upper frequency limit fc2τr≈0.04 (where τr is the rotation time scale) depends weakly on the ratio of magnetic field to particle magnetization strength, whereas fc1 tends to zero when this ratio increases. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Physical Review E American Physical Society (APS)

Separation of two attractive ferromagnetic ellipsoidal particles by hydrodynamic interactions under alternating magnetic field

Preview Only

Separation of two attractive ferromagnetic ellipsoidal particles by hydrodynamic interactions under alternating magnetic field

Abstract

In applications where magnetic particles are used to detect and dose targeted molecules, it is of major importance to prevent particle clustering and aggregation during the capture stage in order to maximize the capture rate. Elongated ferromagnetic particles can be more interesting than spherical ones due to their large magnetic moment, which facilitates their separation by magnets or the detection by optical measurement of their orientation relaxation time. Under alternating magnetic field, the rotational dynamics of elongated ferromagnetic particles results from the balance between magnetic torque that tends to align the particle axis with the field direction and viscous torque. As for their translational motion, it results from a competition between direct magnetic particle-particle interactions and solvent-flow-mediated hydrodynamic interactions. Due to particle anisotropy, this may lead to intricate translation-rotation couplings. Using numerical simulations and theoretical modeling of the system, we show that two ellipsoidal magnetic particles, initially in a head-to-tail attractive configuration resulting from their remnant magnetization, can repel each other due to hydrodynamic interactions when alternating field is operated. The separation takes place in a range of low frequencies fc1<f<fc2. The upper frequency limit fc2τr≈0.04 (where τr is the rotation time scale) depends weakly on the ratio of magnetic field to particle magnetization strength, whereas fc1 tends to zero when this ratio increases.
Loading next page...
 
/lp/aps_physical/separation-of-two-attractive-ferromagnetic-ellipsoidal-particles-by-taPEBp6l9G
Publisher
The American Physical Society
Copyright
Copyright © ©2017 American Physical Society
ISSN
1539-3755
eISSN
550-2376
D.O.I.
10.1103/PhysRevE.95.062611
Publisher site
See Article on Publisher Site

Abstract

In applications where magnetic particles are used to detect and dose targeted molecules, it is of major importance to prevent particle clustering and aggregation during the capture stage in order to maximize the capture rate. Elongated ferromagnetic particles can be more interesting than spherical ones due to their large magnetic moment, which facilitates their separation by magnets or the detection by optical measurement of their orientation relaxation time. Under alternating magnetic field, the rotational dynamics of elongated ferromagnetic particles results from the balance between magnetic torque that tends to align the particle axis with the field direction and viscous torque. As for their translational motion, it results from a competition between direct magnetic particle-particle interactions and solvent-flow-mediated hydrodynamic interactions. Due to particle anisotropy, this may lead to intricate translation-rotation couplings. Using numerical simulations and theoretical modeling of the system, we show that two ellipsoidal magnetic particles, initially in a head-to-tail attractive configuration resulting from their remnant magnetization, can repel each other due to hydrodynamic interactions when alternating field is operated. The separation takes place in a range of low frequencies fc1<f<fc2. The upper frequency limit fc2τr≈0.04 (where τr is the rotation time scale) depends weakly on the ratio of magnetic field to particle magnetization strength, whereas fc1 tends to zero when this ratio increases.

Journal

Physical Review EAmerican Physical Society (APS)

Published: Jun 29, 2017

There are no references for this article.

Sorry, we don’t have permission to share this article on DeepDyve,
but here are related articles that you can start reading right now:

Explore the DeepDyve Library

Search

Query the DeepDyve database, plus search all of PubMed and Google Scholar seamlessly

Organize

Save any article or search result from DeepDyve, PubMed, and Google Scholar... all in one place.

Access

Get unlimited, online access to over 18 million full-text articles from more than 15,000 scientific journals.

Your journals are on DeepDyve

Read from thousands of the leading scholarly journals from SpringerNature, Elsevier, Wiley-Blackwell, Oxford University Press and more.

All the latest content is available, no embargo periods.

See the journals in your area

DeepDyve

Freelancer

DeepDyve

Pro

Price

FREE

$49/month
$360/year

Save searches from
Google Scholar,
PubMed

Create lists to
organize your research

Export lists, citations

Read DeepDyve articles

Abstract access only

Unlimited access to over
18 million full-text articles

Print

20 pages / month

PDF Discount

20% off