Get 20M+ Full-Text Papers For Less Than $1.50/day. Start a 14-Day Trial for You or Your Team.

Learn More →

Impact of antiferromagnetism on the optical properties of rare-earth nickelates

Impact of antiferromagnetism on the optical properties of rare-earth nickelates We study the temperature dependence of the optical conductivity of rare-earth nickelate films of varying composition and strain close to the antiferromagnetic ordering temperature, TN. Two prominent peaks at 0.6 and 1.3 eV, which are characteristic of the insulating phase, display a small but significant increase in intensity when the material passes from para- to antiferromagnetic. This observation indicates the presence of a positive feedback between antiferromagnetic (AF) and bond disproportionation (BD) order. By analyzing the temperature dependence near TN, and using a Landau-type free-energy expression for BD and AF order, we infer that BD order is a necessary condition for the AF phase to appear, and that the antiferromagnetism contributes to stabilization of the bond disproportionation. This model also explains why hysteresis is particularly strong when the transition into the insulating state occurs simultaneously with antiferromagnetic order. http://www.deepdyve.com/assets/images/DeepDyve-Logo-lg.png Physical Review B American Physical Society (APS)

Impact of antiferromagnetism on the optical properties of rare-earth nickelates

Impact of antiferromagnetism on the optical properties of rare-earth nickelates

Physical Review B , Volume 96 (4) – Jul 17, 2017

Abstract

We study the temperature dependence of the optical conductivity of rare-earth nickelate films of varying composition and strain close to the antiferromagnetic ordering temperature, TN. Two prominent peaks at 0.6 and 1.3 eV, which are characteristic of the insulating phase, display a small but significant increase in intensity when the material passes from para- to antiferromagnetic. This observation indicates the presence of a positive feedback between antiferromagnetic (AF) and bond disproportionation (BD) order. By analyzing the temperature dependence near TN, and using a Landau-type free-energy expression for BD and AF order, we infer that BD order is a necessary condition for the AF phase to appear, and that the antiferromagnetism contributes to stabilization of the bond disproportionation. This model also explains why hysteresis is particularly strong when the transition into the insulating state occurs simultaneously with antiferromagnetic order.

Loading next page...
 
/lp/aps_physical/impact-of-antiferromagnetism-on-the-optical-properties-of-rare-earth-5oB05mn1gJ

References

References for this paper are not available at this time. We will be adding them shortly, thank you for your patience.

Publisher
American Physical Society (APS)
Copyright
Copyright © ©2017 American Physical Society
ISSN
1098-0121
eISSN
1550-235X
DOI
10.1103/PhysRevB.96.045120
Publisher site
See Article on Publisher Site

Abstract

We study the temperature dependence of the optical conductivity of rare-earth nickelate films of varying composition and strain close to the antiferromagnetic ordering temperature, TN. Two prominent peaks at 0.6 and 1.3 eV, which are characteristic of the insulating phase, display a small but significant increase in intensity when the material passes from para- to antiferromagnetic. This observation indicates the presence of a positive feedback between antiferromagnetic (AF) and bond disproportionation (BD) order. By analyzing the temperature dependence near TN, and using a Landau-type free-energy expression for BD and AF order, we infer that BD order is a necessary condition for the AF phase to appear, and that the antiferromagnetism contributes to stabilization of the bond disproportionation. This model also explains why hysteresis is particularly strong when the transition into the insulating state occurs simultaneously with antiferromagnetic order.

Journal

Physical Review BAmerican Physical Society (APS)

Published: Jul 17, 2017

There are no references for this article.