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J. Electroanal. Chem. Interfacial Electrochem
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We present high-resolution angle-resolved photoelectron spectroscopy on Au(110). The unreconstructed surface shows a Shockley-type surface state at E 0 = 590 meV whereas on the ( 2 × 1 ) missing-row reconstructed surface no such surface state below E F can be detected. We performed relativistic local-density approximation calculations which agree well with our experimental data. Adsorption of 1 monolayer Ag on the ( 2 × 1 ) reconstructed surface results in a destruction to a ( 1 × 1 ) surface structure and a Shockley state appears at E 0 = 475 meV . Shifting down the surface state from just above to below E F by Na adsorption allowed to extrapolate a binding energy on the reconstructed surface of E 0 = − 120 meV above the Fermi level.
Physical Review B – American Physical Society (APS)
Published: Nov 15, 2008
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