TY - JOUR AU - Yamashita,, Satoru AB - Abstract We have investigated the status of the nuclear fuel assemblies in the Unit-1 reactor of the Fukushima Daiichi nuclear power plant by cosmic muon radiography. In this study, muon tracking detectors were placed outside the reactor building. We succeeded in identifying the inner structure of the reactor complex, such as the reactor containment vessel, pressure vessel, and other structures of the reactor building, through the concrete wall of the reactor building. We found that a large number of fuel assemblies were missing in the original fuel loading zone inside the pressure vessel. The natural interpretation is that most of the nuclear fuel was melted and dropped down to the bottom of the pressure vessel or even below. 1. Introduction The nuclear power reactors of Fukushima Daiichi were heavily damaged by the giant earthquake and subsequent tsunami that occurred in March 2011. Decommissioning of the damaged reactors is taking place. However, before proceeding it is necessary to acquire information about the status of the reactors. Because of the high radiation inside and around the reactor buildings, it is not easy to gain access for close inspection of the reactor status. We proposed using a technique called cosmic muon radiography (CMR) [1,2] to study the current situation of the reactor, specifically the status of the nuclear fuel assemblies. To validate the method we constructed a detector system and evaluated its performance by imaging the nuclear reactor of the JAPC at Tokai, Ibaraki, Japan, using CMR. We successfully imaged the inner structure of the reactor by detecting comic muons penetrating the reactor with the detector placed outside the reactor building [3]. Encouraged by the successful results, and after a study of the on-site radiation level, we carried out CMR imaging of the Unit-1 reactor of Fukushima Daiichi from February 2014 to June 2015. The Unit-1 reactor was damaged with its top concrete walls blown away by a hydrogen gas explosion, as shown in Fig. 1. During our investigation, the whole building was covered to prevent any debris flying out. Details of the investigation are given in this report. Fig. 1. Open in new tabDownload slide Damaged Unit-1 reactor of Fukushima Daiichi, viewed from the north-west side. The Unit-2 building is seen to the right. (Courtesy of TEPCO, the Tokyo Electric Power Company Ltd.) Fig. 1. Open in new tabDownload slide Damaged Unit-1 reactor of Fukushima Daiichi, viewed from the north-west side. The Unit-2 building is seen to the right. (Courtesy of TEPCO, the Tokyo Electric Power Company Ltd.) 2. The muon detection system The detection of cosmic muons was made by X|${-}$|Y sets of 1 cm-wide plastic scintillation bar counters (PSCs) arranged in a plane of 1 m|$\times $|1 m. While we used two X|${-}$|Y sets of the PSC plane for the muon telescope system at the JAPC [3], we used three sets at the Fukushima Daiichi reactor to be robust against possible accidental coincidence due to the environmental high radiation. The muon telescope was housed in a container of 10 cm-thick iron to suppress the effects of the environmental radiation. 2.1. Protection of the detector against the environmental radiation The major concern in operating the detector on-site at Fukushima Daiichi was the effect of the environmental radiation, which was reported to be as high as 0.5 mSv/h around the Unit-1 reactor building. There were also some “hot spots” where the radiation level was much higher. The main components of the environmental radiation were mainly 662 keV gamma rays from Cs|$^{137}$| and gamma rays (mainly 605 and 796 keV) from Cs|$^{154}$|⁠, and their Compton electrons may deteriorate the cosmic muon tracking. We considered shielding the detector with iron, and to evaluate the necessary thickness of the iron shield we performed a “test tracking” with a sample detector placed in a 5 cm-thick iron box. The sample detector was made of three layers of ten PSCs, the same PSCs used for the muon telescope. The iron shield box was additionally surrounded with iron plates of 5 or 10 cm thickness, and therefore we obtained data for iron thicknesses of 5, 10 and 15 cm. Figure 2 shows the sample detector placed in the 5 cm-thick iron shield box. We brought this system near to the Unit-1 reactor building and studied the effect of the environmental radiation on cosmic muon tracking. Fig. 2. Open in new tabDownload slide Left: Sample detector (10 cm wide|$\times $|1 m long|$\times $|10 cm thick) placed in a 5 cm-thick iron shield box. Right: Cross-sectional view of the three-layer sample detector, indicating the grouping of the three layers. Fig. 2. Open in new tabDownload slide Left: Sample detector (10 cm wide|$\times $|1 m long|$\times $|10 cm thick) placed in a 5 cm-thick iron shield box. Right: Cross-sectional view of the three-layer sample detector, indicating the grouping of the three layers. The suppression factors of the gamma rays from Cs|$^{134}$| and Cs|$^{137}$| were estimated by a GEANT simulation as a function the iron thickness, assuming that the gamma rays were normally incident (H. Hirayama, private communication). The gamma yield is expected to be suppressed to 0.3 with 5 cm-thick iron and to 0.03 with 10 cm-thick iron, as shown in Fig. 3. To compare with the simulation results, we first used a handy radiation monitor tightly enclosed in 10 cm-thick iron plates to directly measure the suppression factor at the site planned for deployment of the detector. The measured suppression is close to the 15 cm simulation, as plotted in Fig. 3; the difference can be explained by the average path length in the measured configuration being 13 cm taking into account that the gamma rays are coming from any direction. Fig. 3. Open in new tabDownload slide Suppression factor of the gamma rays from Cs|$^{134}$| and Cs|$^{137}$| estimated by a GEANT simulation as a function of the thickness of the iron, assuming the gamma rays are injected normally to the iron. The value measured on-site for 10 cm of iron is shown by the star. Fig. 3. Open in new tabDownload slide Suppression factor of the gamma rays from Cs|$^{134}$| and Cs|$^{137}$| estimated by a GEANT simulation as a function of the thickness of the iron, assuming the gamma rays are injected normally to the iron. The value measured on-site for 10 cm of iron is shown by the star. The signals of the sample detector were read out by the same system [3] as for the muon telescope where the existence of coincidence hits in two layers is required. For the three-layer sample detector, we assigned the two top layers as “X” and the bottom layer as “Y”, requiring at least one hit in each group of “X” and “Y” (note that all three scintillator bars run in the same direction despite the naming X or Y). Figure 4 shows the “X1–Y” coincidence rates measured on-site at Fukushima Daiichi for the three thicknesses of the iron shield as a function of the width of coincidence time window. As the accidental coincidence increases linearly with the coincidence time window width, the measured rate is affected by the environmental radiation for a time window longer than 100 ns for 5 cm of iron, and started to be affected above 1000 ns for 10 cm of iron. Fig. 4. Open in new tabDownload slide Coincidence rates measured with the test detector as a function of the time window of the coincidence. The data are shown for the three iron thicknesses measured at the Fukushima Daiichi site, and one measured at Yotsukura, about 50 km south. The ambient radiation level at Yotsukura was below 1 |$\mu $|Sv/h. Fig. 4. Open in new tabDownload slide Coincidence rates measured with the test detector as a function of the time window of the coincidence. The data are shown for the three iron thicknesses measured at the Fukushima Daiichi site, and one measured at Yotsukura, about 50 km south. The ambient radiation level at Yotsukura was below 1 |$\mu $|Sv/h. The typical time window we employ for the muon telescope is 16 or 32 ns. This time window needs to be multiplied by a factor 5 to 10 in evaluating the effect in the complete telescope using the present results of the sample detector, since the number of scintillator bars (100 in the complete system) to be considered is greater by this factor. We conclude that the coincidence rate is barely affected for an iron shield thicker than 10 cm. Figure 5 shows the hit position correlation between the “X1” and “Y” layers when exactly one hit is required to be found in each of “X1” and “Y”. As expected, correlation is clearly seen for the 10 cm iron up to a 1024 ns time window. For the 5 cm iron, the correlation is less clear and influenced more by increasing the time window width. The study was repeated for a relaxed threshold setting, 0.8 times the nominal setting, to investigate the effect of the possible uncertainty in the threshold determination, and found a small dependence. Fig. 5. Open in new tabDownload slide X2 and Y hit correlation measured with the test detector; (left) for 10 cm of iron and (right) for a 5 cm iron shield. The results are shown for three typical time window widths, 16, 128, and 1024 ns. Fig. 5. Open in new tabDownload slide X2 and Y hit correlation measured with the test detector; (left) for 10 cm of iron and (right) for a 5 cm iron shield. The results are shown for three typical time window widths, 16, 128, and 1024 ns. Finally, we examined whether we can find a hit in the middle layer X2 when X1 and Y recorded hits at the same channel number. The hit correlations are shown in Fig. 6 for typical cases with 10 and 5 cm iron shield thicknesses. The plots are normalized such that the number of X1=Y events is 1000. X2 hits can be found at the proper position with efficiencies of more than 90% for the 10 cm iron case with a time window of 1024 ns. The observed efficiency is not large for 5 cm iron, although the correlation itself is not much distorted. This can be explained by the fact that the reference Y=X1 is spurious at some fraction and the corresponding X2 was not found as the event is spurious: once the reference is correct, X2 is found correctly. Fig. 6. Open in new tabDownload slide X2 and Y=X1 hit correlation measured with the test detector; (left) for 10 cm of iron and (right) for a 5 cm iron shield. The time window widths are 1024 ns and 64 ns, respectively. The number of events in each column sum is normalized for |$N(Y=X1) = 1000$|⁠. Fig. 6. Open in new tabDownload slide X2 and Y=X1 hit correlation measured with the test detector; (left) for 10 cm of iron and (right) for a 5 cm iron shield. The time window widths are 1024 ns and 64 ns, respectively. The number of events in each column sum is normalized for |$N(Y=X1) = 1000$|⁠. 2.2. The detector system for Unit-1 observation Based on the test measurement data and further considerations, we concluded that there will not be any problem in tracking with 10 cm iron. With 5 cm iron, X–Y hit correlation is distorted in a single X–Y assembly. With 5 cm iron and two X–Y assemblies combined, the signal-to-noise ratio will be improved to about 100 for the nominal threshold setting, but limited to 5 for the relaxed threshold setting (0.8 times the nominal). For the detector system to be deployed for the Unit-1 observation, we selected an iron shield thickness of 10 cm and chose conservatively to install three sets of X–Y assemblies. Figure 7 shows one of the muon telescope systems. The detection system was equipped with an air conditioner to provide a constant temperature inside the iron shield of 20|$\pm $|3|${^\circ}$| for stable operation of the photo-device, a multi-pixel photon counter (MPPC). Fig. 7. Open in new tabDownload slide The muon telescope housed in an iron shield box made of 10 cm iron plates. The relative elevation heights of the three X–Y assemblies are adjusted to target the Unit-1 fuel loading zone. For thermal insulation, 6 cm-thick plastic foam is plastered over the inner wall of the box. The cabinet next to the box houses the air conditioner controller and data network hub for data transfer and communication with the assemblies. The total weight is 20 t. Fig. 7. Open in new tabDownload slide The muon telescope housed in an iron shield box made of 10 cm iron plates. The relative elevation heights of the three X–Y assemblies are adjusted to target the Unit-1 fuel loading zone. For thermal insulation, 6 cm-thick plastic foam is plastered over the inner wall of the box. The cabinet next to the box houses the air conditioner controller and data network hub for data transfer and communication with the assemblies. The total weight is 20 t. The X–Y assemblies used for the study at the JAPC at Tokai were refurbished, repairing dead channel,s and two muon telescope systems were constructed at KEK. They were moved to the Fukushima Daiichi site, and placed in January 2015 at the locations marked by red circles in Fig. 8, which shows a plane view of the Unit-1 reactor. The two systems were placed at WN and NW initially, and one of them was moved to the point N later in the summer. The distance to the reactor center is 36 m for the location WN. Fig. 8. Open in new tabDownload slide A plane view of the Unit-1 reactor of Fukushima Daiichi. The observation of the reactor inner structure was made from the three locations marked by red circles. (Courtesy of TEPCO.) Fig. 8. Open in new tabDownload slide A plane view of the Unit-1 reactor of Fukushima Daiichi. The observation of the reactor inner structure was made from the three locations marked by red circles. (Courtesy of TEPCO.) 2.3. Images of the Unit-1 reactor The observation of cosmic rays started in February 2015. We confirmed that the detection systems were functioning properly in an environment with a radiation level of about 500 |$\mu $|Sv/h. Figure 9 shows the Unit-1 reactor images after 90 days, representing the lateral muon absorption distribution, the observed event rates normalized by those obtained at KEK without obstacles in front. Larger absorption due to heavy objects is illustrated by darkness. Fig. 9. Open in new tabDownload slide Images of the Unit-1 reactor of Fukushima Daiichi after 90 days observed by the muon telescope placed at the (left) WN, (middle) NW, and (right) N points given in Fig. 8. Fig. 9. Open in new tabDownload slide Images of the Unit-1 reactor of Fukushima Daiichi after 90 days observed by the muon telescope placed at the (left) WN, (middle) NW, and (right) N points given in Fig. 8. Figure 10 illustrates the image observed by the muon telescope placed at the WN point with the reactor pressure vessel (RPV) marked with the red dotted line. Figure 11 shows the same image, identifying the facilities in the reactor building. One notices no sign of the existence of heavy materials such as a lump of nuclear fuel in the RPV. A natural interpretation is that the nuclear fuel got melted and dropped from its original position in the RPV. Fig. 10. Open in new tabDownload slide The observed image from the WN point with the reactor pressure vessel marked by the red dotted line. Fig. 10. Open in new tabDownload slide The observed image from the WN point with the reactor pressure vessel marked by the red dotted line. Fig. 11. Open in new tabDownload slide Image of the Unit-1 reactor of Fukushima Daiichi after 90 days observed by the detection system placed at the north-western corner of the reactor building. Fig. 11. Open in new tabDownload slide Image of the Unit-1 reactor of Fukushima Daiichi after 90 days observed by the detection system placed at the north-western corner of the reactor building. The distribution pattern of the muon flux reduction can be translated to the distribution of heavy structures inside the reactor complex, as shown in Fig. 10 for the muon telescope placed at the north-western corner (marked as WN in Fig. 8) of the reactor building. We identified the structures such as (1) the reactor pressure vessel, (2) the reactor containment vessel (RCV), (3) the nuclear fuel storage pool, and (4) the north wall of the reactor building. From the three images, we concluded that no lumps of heavy materials can be seen in the core part of the pressure vessel. This observation can be interpreted as most of the loaded nuclear fuel assemblies having melted and dropped from the loading zone. 3. Estimation of the amount of nuclear fuel left in the RPV of the Unit-1 reactor The amount of heavy materials left in the RPV is crucial information to be investigated with the present detection method. Figure 12 illustrates the structure of the Unit-1 reactor. We defined “side-band” regions and evaluated the amount of material in the “core” region from the amounts of material estimated in the side-band regions. We defined three vertical slice regions, (a), (b1), and (b2), by the dash-dotted vertical lines shown in Fig. 12. Fig. 12. Open in new tabDownload slide Structure of the Unit-1 nuclear reactor of Fukushima Daiichi. The red box represents the fuel loading zone. Fig. 12. Open in new tabDownload slide Structure of the Unit-1 nuclear reactor of Fukushima Daiichi. The red box represents the fuel loading zone. Fig. 13. Open in new tabDownload slide An artistic view of the reactor complex of the Unit-1 reactor with the reactor pressure vessel and the spent fuel storage pool. Fig. 13. Open in new tabDownload slide An artistic view of the reactor complex of the Unit-1 reactor with the reactor pressure vessel and the spent fuel storage pool. The amount of materials through which cosmic muons pass is expressed by the density length, which is defined as the density of materials traversed by the muon multiplied by the muon path length. Specifically, for a given zenith angle |$\theta $|⁠, the muon momentum distribution function |$D\left( {\theta :p} \right)$| is used such that the threshold momentum |$p_{0}$| corresponds to the observed value below which muons cannot pass through the materials to be observed. Namely, we solve the following equation: $$\begin{align*} \int_{p=p_0} D\left(\theta :p\right) dp /\int_{p=1} D\left(\theta :p\right) dp = N_{\it obs}/N_0, \end{align*}$$ where |$N_{\text{obs}}$| and |$N_0$| are number of detected muons and the number expected with no material in front (KEK measurement), respectively, and we set the minimum momentum to |$p $|= 1 GeV. Then the threshold momentum |$p_{0}$| is translated to the material path length from the muon range, where we assume that the material is concrete of 2.5 g/cc density. In the calculation, the cosmic muon momentum distribution |$D\left( {\theta :p} \right)$| is taken from the theoretical calculation by Smith and Duller [4] or from a measurement by the Okayama group [5]. The difference between the two assumptions is assigned as a systematic uncertainty. A more detailed description of the present method is given in the Appendix. The differences of the obtained density-length distribution (a) - (b1) and (a) - (b2) are plotted in Fig. 14. Although the material distributions in these slices are not identical, the possible zenith angle dependence of the muon flux can be diminished by subtraction. In practice, the density length along (b2) is much larger due to the nuclear fuel storage pool located behind the slice of (b2). Therefore, we take only the difference (a) - (b1) to evaluate the amount of material remaining in the fuel loading zone. Fig. 14. Open in new tabDownload slide Left: The density length along the slice (b1) subtracted from that along slice (a). Right: the density length along the slice (b2) subtracted from that along slice (a). The vertical range corresponding to the fuel loading zone is indicated by the shaded box in the figures. Fig. 14. Open in new tabDownload slide Left: The density length along the slice (b1) subtracted from that along slice (a). Right: the density length along the slice (b2) subtracted from that along slice (a). The vertical range corresponding to the fuel loading zone is indicated by the shaded box in the figures. The evaluated amounts in tons are summarized in Table 1. The subtraction results are shown separately for different height ranges, one covering the fuel loading zone, the others underneath and above the loading zone. We independently calculated the weights in the corresponding regions from the engineering drawing of the Unit-1 reactor and obtained 72 tons for the (a) - (b1) weight in the region above the loading zone, while we measured 32|$\pm $|6(stat)|$\pm $|11(syst) tons. The difference is taken as a systematic uncertainty and added conservatively to the amount by taking the different height coverage into account. The amounts shown in row (a) of Table 1 are the resulting values corresponding to the “excess” in slice (a). The systematic uncertainty is composed of the material difference between the measurement and calculation (described above), the difference of the momentum modelling, and the difference of the detector efficiency measured at KEK and on-site at the Unit-1 reactor. Among these, the momentum modelling is the largest. It is larger in the height range underneath the loading zone because the available muon flux data is limited in this zenith angle range. Table 1. Measured amount of material in the RPV for different height regions. Region . 15.2 m < h < 20.3 m . 20.3 m < h < 24.0 m . 24.0 m < h < 31m . . (beneath loading zone) . (loading zone) . (above loading zone) . (a) - (b1) 4|$\pm $|25(stat)|$\pm $|32(syst) tons 1|$\pm $|7(stat)|$\pm $|5(syst) tons 32|$\pm $|6(stat)|$\pm $|11(syst) tons (a) 33|$\pm $|25(stat)|$\pm $|43(syst) tons 22|$\pm $|7(stat)|$\pm $|22(syst) tons 72* Region . 15.2 m < h < 20.3 m . 20.3 m < h < 24.0 m . 24.0 m < h < 31m . . (beneath loading zone) . (loading zone) . (above loading zone) . (a) - (b1) 4|$\pm $|25(stat)|$\pm $|32(syst) tons 1|$\pm $|7(stat)|$\pm $|5(syst) tons 32|$\pm $|6(stat)|$\pm $|11(syst) tons (a) 33|$\pm $|25(stat)|$\pm $|43(syst) tons 22|$\pm $|7(stat)|$\pm $|22(syst) tons 72* *Calculated from the engineering drawing. Open in new tab Table 1. Measured amount of material in the RPV for different height regions. Region . 15.2 m < h < 20.3 m . 20.3 m < h < 24.0 m . 24.0 m < h < 31m . . (beneath loading zone) . (loading zone) . (above loading zone) . (a) - (b1) 4|$\pm $|25(stat)|$\pm $|32(syst) tons 1|$\pm $|7(stat)|$\pm $|5(syst) tons 32|$\pm $|6(stat)|$\pm $|11(syst) tons (a) 33|$\pm $|25(stat)|$\pm $|43(syst) tons 22|$\pm $|7(stat)|$\pm $|22(syst) tons 72* Region . 15.2 m < h < 20.3 m . 20.3 m < h < 24.0 m . 24.0 m < h < 31m . . (beneath loading zone) . (loading zone) . (above loading zone) . (a) - (b1) 4|$\pm $|25(stat)|$\pm $|32(syst) tons 1|$\pm $|7(stat)|$\pm $|5(syst) tons 32|$\pm $|6(stat)|$\pm $|11(syst) tons (a) 33|$\pm $|25(stat)|$\pm $|43(syst) tons 22|$\pm $|7(stat)|$\pm $|22(syst) tons 72* *Calculated from the engineering drawing. Open in new tab The amount of the fuel assemblies originally at the loading zone is estimated to be 160 tons. From the observation described above, we come to the conclusion that most of the nuclear fuel loaded initially at the loading zone in the RPV melted and dropped to the bottom of part of the RPV, or even below, penetrating through to the RCV. Unfortunately, we cannot further detail the status of the fuel debris around the bottom part of the RPV because the cosmic muon flux is limited in the present arrangement of the muon telescope located at the corner of the reactor building. At the location N shown in Fig. 8, the fuel storage pool behind the RPV degrades the measurement. It would be necessary to lower the telescope and set it closer to the RPV so that the bottom part of the reactor can be viewed. 4. Summary We studied the fuel status of the Unit-1 reactor at Fukushima Daiichi using cosmic muon telescope detectors placed outside the reactor building. We succeeded in identifying major stuctures of the reactor complex, reactor containment vessel, pressure vessel, and others. The observed absorption map clearly indicates that heavy material causing significant attenuation of cosmic muons is missing in the fuel loading zone inside the pressure vessel. Our interpretation is that the nuclear fuel assemblies had melted and dropped to the bottom of the pressure vessel or even below. The amounts of material in the fuel loading zone and below were estimated, and the results are consistent with the above conclustion. We tried to detail the bottom part of the pressure vessel in a search for strong attenuation of the cosmic muons; however, no evidence of strong attenuation was identified. To understand this result, two possibilities are considered: (1) the nuclear fuel melted and dropped beyond the scope of the present detector coverage, and (2) the energy of cosmic muons at shallow angles is so high that they penetrate the nuclear debris possibly present at the bottom part of the RPV. We are currently studying whether cosmic rays at shallow elevation angles can penetrate large amounts of materials, therefore we cannot determine the structure of the nuclear reactor in the corresponding angle range by the method employed in this study. Acknowledgements The present study has been carried out as a project supported by the International Research Institute for Nuclear Decommissioning IRID. The cooperation and lots of help provided by TEPCO and Tokyo Power Technology Ltd were essential in the detector installation and operation. We thank Professor Hirotaka Sugawara of the Okinawa Institute of Science and Technology for much advice and many suggestions. Appendix. Derivation of the effective mass of the fuel debris We describe the calculation methods employed to derive the mass of an object from the observed muon transmission. Overall, the muon transmission was defined as the ratio of the flux distributions measured with and without the object in front. The data without the object were collected at KEK or other places where no object was located in front. This method reduces the uncertainty originating from the detector non-uniformity, for example. The nuclear plant building is composed mainly of shielding concrete. Figure A1 illustrates the density-length (density multiplied by the path length) distribution of the Unit-1 nuclear plant viewed from the NW point, which was calculated using the available design drawings. It distributes in the range 30–70 m|$\cdot $|g/cm|$^{3}$| vertically along the axis of the pressure vessel, the target region to be investigated. The density-length range in other views is within 20–80 m|$\cdot $|g/cm|$^{3 }$|and the corresponding minimum muon momenta to pass through are 4–17 GeV/c, calculated based on the continuous slowing down approximation (CSDA) range, see Fig. A2. Fig. A1. Open in new tabDownload slide Density-length distribution (in m|$\cdot $|g/cm3) viewed from the WN point in the plane of the detector view area. The axes are the horizontal and vertical directions of the muon tracks. Fig. A1. Open in new tabDownload slide Density-length distribution (in m|$\cdot $|g/cm3) viewed from the WN point in the plane of the detector view area. The axes are the horizontal and vertical directions of the muon tracks. Fig. A2. Open in new tabDownload slide Correlation between the minimum muon momentum and the muon range. The assumed material is concrete of standard density 2.3 g/cm|$^{3}$|⁠. Fig. A2. Open in new tabDownload slide Correlation between the minimum muon momentum and the muon range. The assumed material is concrete of standard density 2.3 g/cm|$^{3}$|⁠. The view area of the detector, as shown in Fig. A1, is wide enough to cover the pressure vessel (the area to be investigated) and other reactor building structures. The structures can be assumed to be composed of concrete. Therefore the flux data outside the area to be investigated is related to the density-length distribution calculated using the design drawings, as a function of the muon zenith angle. Since the muon momentum is strongly dependent on the zenith angle, this method provides a more reliable estimate than simply relying on the muon momentum distribution projected from the available flux measurement. Also, in the calculation using the projected muon momentum distribution, we would need to assume the flux reduction to be caused by the CSDA range. In the search area, we need to consider any CSDA range difference between the concrete and other materials. Figure A3 plots the calculated CSDA range values as a function of the muon momentum for the typical materials in the search area. It should be noted that the absolute values are not identical but the momentum dependences are similar within |$\pm $|5%. The muon flux reduction should be a function of |$a\rho L$|⁠, where |$a $|is the absorption coefficient related to the CSDA range, |$\rho \mathfrak{g}$|s the density, and |$L$| is the path length. The difference in the absolute values is taken into the systematic uncertainty in |$a$|⁠. Fig. A3. Open in new tabDownload slide Calculated ratio of CSDA range to concrete for the materials abundant in the pressure vessel as a function of the muon momentum. The ratio for UO|$_{2}$| varies from 1.41 to 1.32 (a change of 10%) in the momentum range concerned. Fig. A3. Open in new tabDownload slide Calculated ratio of CSDA range to concrete for the materials abundant in the pressure vessel as a function of the muon momentum. The ratio for UO|$_{2}$| varies from 1.41 to 1.32 (a change of 10%) in the momentum range concerned. The density-length distribution derived from the observed muon flux reduction map are subtracted from the calculated density-length distribution of the structures in the front and in the rear of the search region, namely the pressure vessel. Or the subtraction was conducted using the region next to the search region. The remaining density-length distribution was multiplied by the size of the search area to derive the amount of material left in the pressure vessel. References [1] Nagamine K. , Iwasaki M., Shimomura K., and Ishida K., Nucl. Instrum. Methods Phys. Res. A 356 , 585 ( 1995 ). ( http://dx.doi.org/10.1016/0168-9002(94)01169-9 ) Crossref Search ADS [2] Tanaka H. , Nagamine K., Kawamura N., Nakamura S. N., Ishida K., and Shimomura K., Hyperfine Interact. 138 , 521 ( 2001 ). ( http://dx.doi.org/10.1023/A:1020843100008 ) Crossref Search ADS [3] Fujii H. , et al. , Prog. Theor. Exp. Phys. 2013 , 073C01 ( 2013 ). ( https://doi.org/10.1093/ptep/ptt046 ) Crossref Search ADS [4] Smith J. A. and Duller N. M., J. Geophys. Res. 64 , 2297 ( 1959 ). ( http://dx.doi.org/10.1029/JZ064i012p02297 ) Crossref Search ADS [5] Tsuji S. , Ph.D. thesis , Okayama University ( 1998 ) [in Japanese]; available at http://ousar.lib.okayama-u.ac.jp/ja/8238. © The Author(s) 2020. Published by Oxford University Press on behalf of the Physical Society of Japan. This is an Open Access article distributed under the terms of the Creative Commons Attribution License (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted reuse, distribution, and reproduction in any medium, provided the original work is properly cited. TI - Investigation of the Unit-1 nuclear reactor of Fukushima Daiichi by cosmic muon radiography JF - Progress of Theoretical and Experimental Physics DO - 10.1093/ptep/ptaa027 DA - 2020-04-01 UR - https://www.deepdyve.com/lp/oxford-university-press/investigation-of-the-unit-1-nuclear-reactor-of-fukushima-daiichi-by-QgrDwXyY1M VL - 2020 IS - 4 DP - DeepDyve ER -