TY - JOUR AU1 - Yin, Zhuoxin AU2 - Pan, Duoqiang AU3 - Li, Ping AU4 - Liu, Peng AU5 - Wu, Hanyu AU6 - Wu, Wangsuo AB - AbstractThe sorption of hexavalent uranium on muscovite as a function of pH, background electrolyte, temperature and humic acid (HA) was investigated in detail using batch experiments. The results showed that the uranium sorpiton on muscovite was kinetic fast, the kinetic process was fitted well by pseudo-second-order kinetic model. The sorption of uranium depended strongly on pH while weakly on background electrolyte concentration, indicating that surface complexation dominated the sorption process. The escalation of temperature and humic acid concentration were favorable to uranium sorption on muscovite. The sorption isotherms at pH 6.0 could be described better by Langmuir model than Freundlich or Dubinin-Radushkevich (D-R) model, thermodynamic data indicated that the uranium sorption process on muscovite was spontaneous and endothermic process. The findings in present work can provide important experimental reference for understanding the environmental behavior of uranium in mica-rich terrains. TI - Retardation of hexavalent uranium in muscovite environment: a batch study JF - Radiochimica Acta DO - 10.1515/ract-2017-2888 DA - 2018-07-26 UR - https://www.deepdyve.com/lp/de-gruyter/retardation-of-hexavalent-uranium-in-muscovite-environment-a-batch-PwrmYyBO46 SP - 559 EP - 567 VL - 106 IS - 7 DP - DeepDyve ER -