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The title compound, C6H6N4S4, is formed through the thionato S-S bonding of parent 2-mercapto-5-methyl-1,3,4-thiadiazole molecules, following the deprotonation of thiol groups in a mixed solvent. The title compound crystallizes in the monoclinic system, space group C2/c. The S-S distance is 2.028...