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- Publisher
- Springer Journals
- Copyright
- Copyright © Springer 1991
- ISSN
- 0922-6168
- eISSN
- 1568-5675
- DOI
- 10.1163/156856791x00057
- Publisher site
- See Article on Publisher Site
Abstract
Research on Chemical Intermediates, 15 ( 1991 ) 165-182 165 Elsevier Science Publishers B.V., Amsterdam STRUCTURE AND REACTIVITY OF SILICA-SUPPORTED VANADIUM OXIDE S. TED OYAMA Departments of Chemical Engineering and Chemistry Clarkson University Potsdam, New York 13699-5705 USA CONTENTS I. Introduction .................................................................................................................. 166 I1. Structure of Silica-Supported Vanadium Oxide ..................................................... : 166 A. General considerations ................................................................................... 166 B. Ambient condition studies .............................................................................. 167 C. Controlled atmosphere studies ...................................................................... 169 III. Reactivity of the Surface Vanadium Oxide Species ............................................... 171 IV. Quantitation of the Active Vanadia Surface ............................................................ 173 V. Catalytic Activity of Supported Vanadium Oxide ................................................... 173 A. Photooxidation ofpropene and carbon monoxide ...................................... 173 B. Photoisomerization and photooxidation of butenes ................................... 174 C. Hydroxylation with N20 of benzene and methane ................................... 175 D. Oxidation of tetrahydrofuran ......................................................................... 175 E. Oxidative scission of butane ........................................................................... 176 E Oxidation of 1-butene ..................................................................................... 176 G. Oxidation ofpropene ....................................................................................... 177 H. Oxidation ofethanot ........................................................................................ 177 I. Oxidation ofethane ........................................................................................ 178 VI. Influence of Mode of Adsorbate Bonding on Selectivity ..................................... 178 VII. Acknowledgement ...................................................................................................... 179 VIII. References .................................................................................................................... 179 0922-6168/91/$03.50 9 1991 -- Elsevier Science Publishers B.V. 166 I. INTRODUCTION Vanadium oxide is a key component in a number of widely used
Journal
Research on Chemical Intermediates – Springer Journals
Published: Jun 1, 1991
Keywords: Vanadium; Acrolein; Vanadium Oxide; Ethanol Oxidation; Oxygen Chemisorption